GaSe crystals
Using a GaSe crystal the output wavelength was tuned in the range of from 58.2 µm to 3540 µm (from 172 cm-1 to 2.82 cm-1) with the peak power reaching 209 W. Significantly improved was made to the output power of this THz source from 209 W to 389 W.
ZnGeP2 crystals
On the other hand, based on DFG in a ZnGeP2 crystal the output wavelength was tuned in the ranges of 83.1–1642 µm and 80.2–1416 µm for two phase matching configurations, respectively.The output power has reached 134 W.
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GaP crystals
Using a GaP crystal the output wavelength was tuned in the range of 71.1−2830 µm whereas the highest peak power was 15.6 W.The advantage of using GaP over GaSe and ZnGeP2 is obvious: crystal rotation is no longer required for achieving wavelength tuning.Instead, one just needs to tune the wavelength of one mixing beam within a bandwidth of as narrow as 15.3 nm.
To summary
The conversion efficiency of 0.1% is also the highest ever achieved for a tabletop system using a commercially-available laser system as the pump sources.The only THz source that could compete with GaSe THz source is a free-electron laser, which is extremely bulky and consumes a huge electrical power. Furthermore, the output wavelengths of thisTHz sources can be tuned in extremely-wide ranges, unlike the quantum cascade lasers each of which can only generate a fixed wavelength.Therefore, certain applications which can be realized using widely-tunable monochromatic THz sources would not be possible if relying on the subpicosecond THz pulses or quantum cascade lasers instead.